Evolution of the functionalities and structures of biochar in pyrolysis of poplar in a wide temperature range.
Identifieur interne : 000412 ( Main/Exploration ); précédent : 000411; suivant : 000413Evolution of the functionalities and structures of biochar in pyrolysis of poplar in a wide temperature range.
Auteurs : Chenting Zhang [République populaire de Chine] ; Zhanming Zhang [République populaire de Chine] ; Lijun Zhang [République populaire de Chine] ; Qingyin Li [République populaire de Chine] ; Cuncheng Li [République populaire de Chine] ; Guozhu Chen [République populaire de Chine] ; Shu Zhang [République populaire de Chine] ; Qing Liu [République populaire de Chine] ; Xun Hu [République populaire de Chine]Source :
- Bioresource technology [ 1873-2976 ] ; 2020.
Descripteurs français
- KwdFr :
- MESH :
English descriptors
- KwdEn :
- MESH :
- chemical : Charcoal.
- Hot Temperature, Populus, Pyrolysis, Temperature.
Abstract
This study studied the change of functionalities in the biochar formed in pyrolysis of poplar wood in a wide range of temperature. The in situ Diffuse Reflectance Infrared Fourier transform spectroscopy characterization indicated that aldehydes and ketones functionalities formation initiated at 100 °C, dominated at 300 to 500 °C. Carboxyl group was less stable than carbonyls. Cellulose crystal in poplar decomposed slightly at 300 °C and significantly at 350 °C. The temperature from 250 to 350 °C significantly affected biochar yields, while the drastic fusion of the ring structures in biochar occurred from 550 to 650 °C, making biochar more aliphatic while less more aromatic. High pyrolysis temperature also created more defective structures in the biochar and favored the absorption of the CO2 generated during the pyrolysis. The results provide the reference information for understanding the structural configuration and evolution of the functionalities during in pyrolysis of poplar biomass.
DOI: 10.1016/j.biortech.2020.123002
PubMed: 32078904
Affiliations:
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in pyrolysis of poplar in a wide temperature range.</title><author><name sortKey="Zhang, Chenting" sort="Zhang, Chenting" uniqKey="Zhang C" first="Chenting" last="Zhang">Chenting Zhang</name><affiliation wicri:level="1"><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Material Science and Engineering, University of Jinan, Jinan 250022</wicri:regionArea><wicri:noRegion>Jinan 250022</wicri:noRegion></affiliation></author><author><name sortKey="Zhang, Zhanming" sort="Zhang, Zhanming" uniqKey="Zhang Z" first="Zhanming" last="Zhang">Zhanming Zhang</name><affiliation wicri:level="1"><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Material Science and Engineering, University of Jinan, Jinan 250022</wicri:regionArea><wicri:noRegion>Jinan 250022</wicri:noRegion></affiliation></author><author><name sortKey="Zhang, Lijun" sort="Zhang, Lijun" uniqKey="Zhang L" first="Lijun" last="Zhang">Lijun Zhang</name><affiliation wicri:level="1"><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Material Science and Engineering, University of Jinan, Jinan 250022</wicri:regionArea><wicri:noRegion>Jinan 250022</wicri:noRegion></affiliation></author><author><name sortKey="Li, Qingyin" sort="Li, Qingyin" uniqKey="Li Q" first="Qingyin" last="Li">Qingyin Li</name><affiliation wicri:level="1"><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Material 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Chine</country><wicri:regionArea>School of Chemistry and Chemical Engineering, University of Jinan, Jinan 250022</wicri:regionArea><wicri:noRegion>Jinan 250022</wicri:noRegion></affiliation></author><author><name sortKey="Zhang, Shu" sort="Zhang, Shu" uniqKey="Zhang S" first="Shu" last="Zhang">Shu Zhang</name><affiliation wicri:level="1"><nlm:affiliation>College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037</wicri:regionArea><wicri:noRegion>Nanjing 210037</wicri:noRegion></affiliation></author><author><name sortKey="Liu, Qing" sort="Liu, Qing" uniqKey="Liu Q" first="Qing" last="Liu">Qing Liu</name><affiliation wicri:level="1"><nlm:affiliation>Key Laboratory of Low Carbon Energy and Chemical Engineering, College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, PR China.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Key Laboratory of Low Carbon Energy and Chemical Engineering, College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590</wicri:regionArea><wicri:noRegion>Qingdao 266590</wicri:noRegion></affiliation></author><author><name sortKey="Hu, Xun" sort="Hu, Xun" uniqKey="Hu X" first="Xun" last="Hu">Xun Hu</name><affiliation wicri:level="1"><nlm:affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China. Electronic address: xun.hu@outlook.com.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>School of Material Science and Engineering, University of Jinan, Jinan 250022</wicri:regionArea><wicri:noRegion>Jinan 250022</wicri:noRegion></affiliation></author></analytic><series><title level="j">Bioresource technology</title><idno type="eISSN">1873-2976</idno><imprint><date when="2020" type="published">2020</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Charcoal (MeSH)</term><term>Hot Temperature (MeSH)</term><term>Populus (MeSH)</term><term>Pyrolysis (MeSH)</term><term>Temperature (MeSH)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Charbon de bois (MeSH)</term><term>Populus (MeSH)</term><term>Pyrolyse (MeSH)</term><term>Température (MeSH)</term><term>Température élevée (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" xml:lang="en"><term>Charcoal</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Hot Temperature</term><term>Populus</term><term>Pyrolysis</term><term>Temperature</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Charbon de bois</term><term>Populus</term><term>Pyrolyse</term><term>Température</term><term>Température élevée</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">This study studied the change of functionalities in the biochar formed in pyrolysis of poplar wood in a wide range of temperature. The in situ Diffuse Reflectance Infrared Fourier transform spectroscopy characterization indicated that aldehydes and ketones functionalities formation initiated at 100 °C, dominated at 300 to 500 °C. Carboxyl group was less stable than carbonyls. Cellulose crystal in poplar decomposed slightly at 300 °C and significantly at 350 °C. The temperature from 250 to 350 °C significantly affected biochar yields, while the drastic fusion of the ring structures in biochar occurred from 550 to 650 °C, making biochar more aliphatic while less more aromatic. High pyrolysis temperature also created more defective structures in the biochar and favored the absorption of the CO<sub>2</sub> generated during the pyrolysis. The results provide the reference information for understanding the structural configuration and evolution of the functionalities during in pyrolysis of poplar biomass.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Automated" Owner="NLM"><PMID Version="1">32078904</PMID><DateCompleted><Year>2020</Year><Month>03</Month><Day>12</Day></DateCompleted><DateRevised><Year>2020</Year><Month>03</Month><Day>12</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1873-2976</ISSN><JournalIssue CitedMedium="Internet"><Volume>304</Volume><PubDate><Year>2020</Year><Month>May</Month></PubDate></JournalIssue><Title>Bioresource technology</Title><ISOAbbreviation>Bioresour Technol</ISOAbbreviation></Journal><ArticleTitle>Evolution of the functionalities and structures of biochar in pyrolysis of poplar in a wide temperature range.</ArticleTitle><Pagination><MedlinePgn>123002</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0960-8524(20)30271-6</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.biortech.2020.123002</ELocationID><Abstract><AbstractText>This study studied the change of functionalities in the biochar formed in pyrolysis of poplar wood in a wide range of temperature. The in situ Diffuse Reflectance Infrared Fourier transform spectroscopy characterization indicated that aldehydes and ketones functionalities formation initiated at 100 °C, dominated at 300 to 500 °C. Carboxyl group was less stable than carbonyls. Cellulose crystal in poplar decomposed slightly at 300 °C and significantly at 350 °C. The temperature from 250 to 350 °C significantly affected biochar yields, while the drastic fusion of the ring structures in biochar occurred from 550 to 650 °C, making biochar more aliphatic while less more aromatic. High pyrolysis temperature also created more defective structures in the biochar and favored the absorption of the CO<sub>2</sub> generated during the pyrolysis. The results provide the reference information for understanding the structural configuration and evolution of the functionalities during in pyrolysis of poplar biomass.</AbstractText><CopyrightInformation>Copyright © 2020 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Chenting</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Zhanming</ForeName><Initials>Z</Initials><AffiliationInfo><Affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Lijun</ForeName><Initials>L</Initials><AffiliationInfo><Affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Li</LastName><ForeName>Qingyin</ForeName><Initials>Q</Initials><AffiliationInfo><Affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Li</LastName><ForeName>Cuncheng</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>School of Chemistry and Chemical Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Chen</LastName><ForeName>Guozhu</ForeName><Initials>G</Initials><AffiliationInfo><Affiliation>School of Chemistry and Chemical Engineering, University of Jinan, Jinan 250022, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Shu</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>College of Materials Science and Engineering, Nanjing Forestry University, Nanjing 210037, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Liu</LastName><ForeName>Qing</ForeName><Initials>Q</Initials><AffiliationInfo><Affiliation>Key Laboratory of Low Carbon Energy and Chemical Engineering, College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, PR China.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Hu</LastName><ForeName>Xun</ForeName><Initials>X</Initials><AffiliationInfo><Affiliation>School of Material Science and Engineering, University of Jinan, Jinan 250022, PR China. Electronic address: xun.hu@outlook.com.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2020</Year><Month>02</Month><Day>12</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Bioresour Technol</MedlineTA><NlmUniqueID>9889523</NlmUniqueID><ISSNLinking>0960-8524</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="C540010">biochar</NameOfSubstance></Chemical><Chemical><RegistryNumber>16291-96-6</RegistryNumber><NameOfSubstance UI="D002606">Charcoal</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D002606" MajorTopicYN="N">Charcoal</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D006358" MajorTopicYN="N">Hot Temperature</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D032107" MajorTopicYN="Y">Populus</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D000077319" MajorTopicYN="Y">Pyrolysis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D013696" MajorTopicYN="N">Temperature</DescriptorName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Functionalities of biochar</Keyword><Keyword MajorTopicYN="N">Properties of biochar</Keyword><Keyword MajorTopicYN="N">Pyrolysis of poplar</Keyword><Keyword MajorTopicYN="N">Pyrolysis temperature</Keyword></KeywordList><CoiStatement>Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.</CoiStatement></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2019</Year><Month>12</Month><Day>29</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2020</Year><Month>02</Month><Day>07</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2020</Year><Month>02</Month><Day>08</Day></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2020</Year><Month>2</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2020</Year><Month>3</Month><Day>13</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2020</Year><Month>2</Month><Day>21</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">32078904</ArticleId><ArticleId IdType="pii">S0960-8524(20)30271-6</ArticleId><ArticleId IdType="doi">10.1016/j.biortech.2020.123002</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>République populaire de Chine</li></country></list><tree><country name="République populaire de Chine"><noRegion><name sortKey="Zhang, Chenting" sort="Zhang, Chenting" uniqKey="Zhang C" first="Chenting" last="Zhang">Chenting Zhang</name></noRegion><name sortKey="Chen, Guozhu" sort="Chen, Guozhu" uniqKey="Chen G" first="Guozhu" last="Chen">Guozhu Chen</name><name sortKey="Hu, Xun" sort="Hu, Xun" uniqKey="Hu X" first="Xun" last="Hu">Xun Hu</name><name sortKey="Li, Cuncheng" sort="Li, Cuncheng" uniqKey="Li C" first="Cuncheng" last="Li">Cuncheng Li</name><name sortKey="Li, Qingyin" sort="Li, Qingyin" uniqKey="Li Q" first="Qingyin" last="Li">Qingyin Li</name><name sortKey="Liu, Qing" sort="Liu, Qing" uniqKey="Liu Q" first="Qing" last="Liu">Qing Liu</name><name sortKey="Zhang, Lijun" sort="Zhang, Lijun" uniqKey="Zhang L" first="Lijun" last="Zhang">Lijun Zhang</name><name sortKey="Zhang, Shu" sort="Zhang, Shu" uniqKey="Zhang S" first="Shu" last="Zhang">Shu Zhang</name><name sortKey="Zhang, Zhanming" sort="Zhang, Zhanming" uniqKey="Zhang Z" first="Zhanming" last="Zhang">Zhanming Zhang</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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